Berthier, Ludovic, et al. “A Random Walk Description of the Heterogeneous Glassy Dynamics of Attracting Colloids”. Journal of Physics: Condensed Matter, vol. 20, no. 24, 2008, p. 244126, https://doi.org/10.1088/0953-8984/20/24/244126.

Genre

  • Journal Article
Contributors
Author: Berthier, Ludovic
Author: Chaudhuri, Pinaki
Author: Gao, Yongxiang
Author: Kob, Walter
Author: Kilfoil, Maria
Date Issued
2008
Date Published Online
2008-05-29
Abstract

We study the heterogeneous dynamics of attractive colloidal particles close to the gel transition using confocal microscopy experiments combined with a theoretical statistical analysis. We focus on single particle dynamics and show that the self-part of the van Hove distribution function is not the Gaussian expected for a Fickian process, but that it reflects instead the existence, at any given time, of colloids with widely different mobilities. Our confocal microscopy measurements can be described well by a simple analytical model based on a conventional continuous time random walk picture, as already found for several other glassy materials. In particular, the theory successfully accounts for the presence of broad tails in the van Hove distributions that exhibit exponential, rather than Gaussian, decay at large distance.

Language

  • English
Page range
244126
Host Title
Journal of Physics: Condensed Matter
Host Abbreviated Title
J. Phys.: Condens. Matter
Volume
20
Issue
24
ISSN
0953-8984
1361-648X

Department